By Ruijun Hou
This thesis bargains novel equipment for catalyst and strategy layout for the selective hydrogenation of acetylene and 1,3-butadiene. the writer predicts the homes of supported Pd–Ni bimetallic catalysts utilizing density sensible idea (DFT) calculations and temperature-programmed desorption (TPD). the wonderful correlation among version surfaces and supported catalysts demonstrates the feasibility of designing potent bimetallic catalysts for selective hydrogenation reactions. the writer additionally proposes a mode for designing non-precious steel catalysts to switch worthwhile metals. she changes the method of selective hydrogenation of acetylene through coupling the selective adsorption to the selective hydrogenation within the liquid part, because of which the ethylene selectivity is tremendously better and warmth move is enormously more suitable. finally, via studying the mechanism of liquid-phase hydrogenation, the writer proposes a multi-stage slurry mattress reactor for commercial applications.<
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Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene (Springer Theses) by Ruijun Hou